HIGHLIGHTS
SUMMARY
Using a site-by-site approach at low temperature to visualize the reaction pathway, the authors find that reactants bond to the Fe-tpy active_sites via surface-bound intermediates, and investigate the role of the substrate in understanding and designing single-site catalysts on metallic supports. Topographic STM images show differences between the bare tpy (Fig 1a left, blue circle indicator) and Fe-coordinated tpy (Fig 1a right, red 4-point star, and Fig 1d, both ends). Preparation and characterization of active Fe-terpyridine site Nature Communications | 13:7407 samples containing active_sites and gaseous . . .
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