HIGHLIGHTS
SUMMARY
It`s expected that the LiPON-based thin-film solid electrolyte can stabilize both the cathode and anode interface and Li-S systems can be well transferred into the untrodden zone of TFBs. In this work, for the first time, TFLSBs were successfully created by stacking VGs-Li2S composite thin-film cathode, LiPON thin-film solid electrolyte, and Li anode. The excellent electrochemical durability of VGs-Li2S composite thin-film cathode for 3,000 cycles is attributed to the favorable compatibility and outstanding interfacial stability between thin-film solid electrolyte with VGs-Li2S composite . . .
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