HIGHLIGHTS
SUMMARY
On the other side, the present author and his group have long been studying the chemical dynamics ranging from nuclear classical and semiclassical dynamics (see ref and more cited there) to full quantum electron dynamics. Preparing beforehand an electronically excited_state of H-Ċ=Ċ-H (bent structure and longer C-C distances, double bond), they de-excited it to the high vibrational excited_state on the electronic ground_state by induced emission. Reflecting the highly vibrational excited_states of polyatomic molecule, the attained spectra were extremely complicated, manifesting the chaotic feature behind. As a candidate among molecules . . .
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